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However, in state-of-the-art devices, performance remains limited by an ineffective hole-transport layer, stemming from the difficulty of controllably and substantially inducing p-type doping in PbS quantum dots. <br>\nHere, we report a method to obtain PbS CQDs with a chalcogenide-rich stoichiometry using organoselenide ligands such as potassium selenocyanate, benzeneselenol, and 1-hydroselenopropan-2-ol, where the weak Se–C bonds of the ligands dissociate under mild annealing, leaving a Se-passivated CQD surface. All resulting CQD thin films exhibit significantly enhanced hole mobilities, when compared to state-of-the-art p-type PbS films, reaching a record of 0.15 cm2 V-1 s-1 using the benzeneselenol ligand. Spectroscopic and computational investigations of 1-seleno-2-propanol-capped CQDs provide strong evidence that the controlled Se–C cleavage enables the chalcogen-rich surface stoichiometry, thereby shifting the Fermi level towards the HOMO level, determining an enhanced p-type behavior. Finally, we utilized this stable selenol-based CQD ink for the scalable fabrication of photodiodes, achieving devices with sensitivity up to 1350 nm, with 374 kHz bandwidth, 80% external quantum efficiency, and an outstanding detectivity of 7.1×1012 Jones. \n<br>\nThis work introduces selenol-based stoichiometry control as a powerful, robust, and generalizable approach to boost carrier transport and device performance in PbS CQD optoelectronics."},"dsDescriptionDate":{"typeName":"dsDescriptionDate","multiple":false,"typeClass":"primitive","value":"2026-04-28"}}]},{"typeName":"subject","multiple":true,"typeClass":"controlledVocabulary","value":["Chemistry","Physics"]},{"typeName":"keyword","multiple":true,"typeClass":"compound","value":[{"keywordValue":{"typeName":"keywordValue","multiple":false,"typeClass":"primitive","value":"lead sulfide quantum dot"}},{"keywordValue":{"typeName":"keywordValue","multiple":false,"typeClass":"primitive","value":"selenol 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